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Grigoriy Sereda Taejin Kim Aubrey Jones Hari Khatri Christopher L. Marshall H. Subramanian Ranjit T. Koodali 《Catalysis Letters》2011,141(8):1086-1096
Abstract
Catalytic performance of solid supported monovanadate catalysts toward oxidation of propane is significantly affected by the templating effect of: (1) pretreatment of the solid support with calixarene derivatives before deposition of ammonium vanadate, (2) direct deposition of vanadyl phthalocyanine as the vanadate precursor. This effect is believed to be linked to the accessibility of the active sites, and was studied in comparison with a reference mesoporous support. 相似文献43.
It is difficult to convey the accelerating rate and growing importance of mass spectrometry applications to human blood proteins and peptides. Mass spectrometry can rapidly detect and identify the ionizable peptides from the proteins in a simple mixture and reveal many of their post‐translational modifications. However, blood is a complex mixture that may contain many proteins first expressed in cells and tissues. The complete analysis of blood proteins is a daunting task that will rely on a wide range of disciplines from physics, chemistry, biochemistry, genetics, electromagnetic instrumentation, mathematics and computation. Therefore the comprehensive discovery and analysis of blood proteins will rank among the great technical challenges and require the cumulative sum of many of mankind's scientific achievements together. A variety of methods have been used to fractionate, analyze and identify proteins from blood, each yielding a small piece of the whole and throwing the great size of the task into sharp relief. The approaches attempted to date clearly indicate that enumerating the proteins and peptides of blood can be accomplished. There is no doubt that the mass spectrometry of blood will be crucial to the discovery and analysis of proteins, enzyme activities, and post‐translational processes that underlay the mechanisms of disease. At present both discovery and quantification of proteins from blood are commonly reaching sensitivities of ~1 ng/mL. © 2010 Wiley Periodicals, Inc., Mass Spec Rev 30:685–732, 2011 相似文献
44.
Hazel Morton Nancie Gunson Diarmid Marshall Fergus McInnes Andrea Ayres Mervyn Jack 《Computer Speech and Language》2011,25(2):341-362
This paper describes a comprehensive usability evaluation of an automated telephone banking system which employs text-to-speech (TTS) synthesis in offering additional detail on customers’ account transactions. The paper describes a series of four experiments in which TTS was employed to offer an extra level of detail to recent transactions listings within an established banking service which otherwise uses recorded speech from a professional recording artist. Results from the experiments show that participants welcome the added value of TTS in being able to provide additional detail on their account transactions, but that TTS should be used minimally in the service. 相似文献
45.
S.P. Marshall S. Taylor C.R. Stone T.J. Davies R.F. Cracknell 《Combustion and Flame》2011,(10):1920-1932
The laminar burning velocity is a fundamental property of a fuel that affects many aspects of its combustion behaviour. Experimental values are required to validate kinetic simulations, and also to provide input for models of flashback, minimum ignition energy and turbulent combustion.A constant volume vessel (rated at 3.4 MPa) in conjunction with a multi-zone model was used to calculate burning velocity from pressure and schlieren data, allowing the user to select data uncorrupted by heat transfer or cellularity. Using the pressure rise data allows measurements to be derived for much higher pressures and temperatures than when the constant pressure data are used. A 12 term correlation for burning velocity was fitted to the data.n-Heptane, iso-octane, toluene, ethylbenzene and ethanol were tested over a wide range of initial pressures (50, 100, 200 and 400 kPa), temperatures (310, 380 and 450 K) and equivalence ratios (0.7–1.4), along with tests using combustion residuals at mole fractions of up to 0.3. The results compared favourably with the limited data already published, especially at high pressures. Conditions at the onset of cellularity are given for iso-octane. 相似文献
46.
Julie K. Furmick Dr. Ichiro Kaneko Angela N. Walsh Joanna Yang Jaskaran S. Bhogal Geoffrey M. Gray Juan C. Baso Drew O. Browder Jessica L. S. Prentice Luis A. Montano Chanh C. Huynh Lisa M. Marcus Dorian G. Tsosie Jungeun S. Kwon Alexis Quezada Nicole M. Reyes Brittney Lemming Puneet Saini Dr. Arjan van der Vaart Dr. Thomas L. Groy Dr. Pamela A. Marshall Dr. Peter W. Jurutka Dr. Carl E. Wagner 《ChemMedChem》2012,7(9):1551-1566
47.
A. Aguilar-Arevalo M. Blecher D.A. Bryman J. Comfort J. Doornbos L. Doria A. Hussein N. Ito S. Kettell L. Kurchaninov C. Malbrunot G.M. Marshall T. Numao R. Poutissou A. Sher B. Walker K. Yamada 《Nuclear instruments & methods in physics research. Section A, Accelerators, spectrometers, detectors and associated equipment》2009,609(2-3):102-105
An extension of the TRIUMF M13 low-energy pion channel designed to suppress positrons based on an energy-loss technique is described. A source of beam channel momentum calibration from the decay π+→e+ν is also described. 相似文献
48.
Researchers and practitioners have long utilized a variety of penetrometers to investigate the snowpack. Identifying definitive relationships between penetrometer-derived microstructural information and stability has been challenging. The purpose of this study is two-fold: 1. We propose a simple field test to establish relationships between load and penetrometer-derived microstructural estimates, 2. We utilize the SnowMicroPen (SMP) to quantify changes in weak layer residual strength and microstructural dimension associated with an artificial loading event. Our dataset is from Moonlight Basin, Montana and includes three modified loaded-column tests, each paired with 5 SMP profiles. Depth hoar comprised the targeted weak layer. Results indicate that loading caused the residual strength and rupture frequency to decrease significantly. Much like a compression test at a micro-scale, the force required for the SMP to rupture individual structures as well as the micro-scale strength decreased significantly when the slab stress was increased by artificially adding blocks of snow. A decrease in observed rupture frequency within the weak layer (or an increase in the distance between ruptured structures) also occurred after the loading event, probably because some structures within the weak layer had already failed or were so close to failing that the penetrometer could not detect their rupture. Due in part to the large difference in loads, microstructural differences between the natural and loaded columns were significant enough that only one profile would have been necessary to determine a significant difference in residual strength. Artificial removal of slab stress resulted in greater rupture forces and larger microstructures, likely due to elastic rebound. 相似文献
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